A Butterfly-Inspired Hierarchical Light-Trapping Structure towards a High-Performance Polarization-Sensitive Perovskite Photodetector

Zhan, Wang, Cheng, Li, Li, Li, Peng, Lu, Wang, Song, Jiang, Li (2019) A Butterfly-Inspired Hierarchical Light-Trapping Structure towards a High-Performance Polarization-Sensitive Perovskite Photodetector Angew Chem Int Ed Engl (IF: -1) 58(46) 16456-16462

Abstract

Extensive applications for photodetectors have led to demand for high-responsivity polarization-sensitive light detection. Inspired by the elaborate architecture of butterfly Papilio paris, a 1D nanograting bonded porous 2D photonic crystal perovskite photodetector (G-PC-PD) using a commercial DVD master and 2D crystalline colloidal arrays template was fabricated. The coupling effect from grating diffraction and reflection of the PC stopband renders the enhanced light harvesting of G-PC-PD. The porous scaffold and nanoimprinting process afford a highly crystalline perovskite film. White light responsivity and detectivity of G-PC-PD are up to 12.67 A W-1 and 3.22×1013  Jones (6∼7 times that of a pristine perovskite photodetector). The highly ordered nanograting arrays of G-PC-PD enable polarization-sensitive light detection with a rate of -0.72 nA deg-1 . This hierarchical perovskite integrated nanograting and 2D PC architecture opens a new avenue to high-performance optoelectronic devices.© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Links

http://www.ncbi.nlm.nih.gov/pubmed/31441973
http://dx.doi.org/10.1002/anie.201908743

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